Single Molecule Imaging Spectroscopy And Nanomanipulation Of Biomolecules In Aqueous Solution

T. Yanagida

Yanagida Biomotron Project, JRDC, Mino, Osaka, Japan.

We have refined total internal reflection fluorescence microscopy (TIRFM) to visualize single fluorescent dye molecules in aqueous solution at a full video rate. This new fluorescence microscopy allowed us to directly image individual ATPase reactions and motions by a single motor protein (Nature, 374, 555- '95; Nature, 380, 451-'96). Furthermore, we have extended this method to single molecule spectroscopy and FRET. Using the single molecule spectroscopy and FRET, we could directly monitor subunit dynamics in a single Ca-binding protein and protein-protein communication at a single molecule level (BS(US), Abs.'97). Combining this method for single molecule imaging with manipulation of a single molecule by laser trapping nanometry, we have succeeded in simultaneous measurements of single molecule mechanics and the ATPase reaction by a motor protein (BS(US), Abs.'97). We are applying these new methods to studies on mechnaochemical energy transduction in molecular motors, DNA -protein interaction and signal transduction in cell.

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